Publications
MoS2 pixel arrays for real-time photoluminescence imaging of redox molecules
Measuring the behavior of redox-active molecules in space and time is crucial for understanding chemical and biological systems and for developing new technologies. Optical schemes are noninvasive and scalable, but usually have a slow response compared to electrical detection methods. Furthermore, many fluorescent molecules for redox detection degrade in brightness over long exposure times. Here, we show that the photoluminescence of “pixel” arrays of monolayer MoS2 can image spatial and temporal changes in redox molecule concentration.
Resolution and dose dependence of radiation damage in biomolecular systems
The local Fourier-space relation between diffracted intensity I, diffraction wavevector q and dose D, , is key to probing and understanding radiation damage by X-rays and energetic particles in both diffraction and imaging experiments. The models used in protein crystallography for the last 50 years provide good fits to experimental I(q) versus nominal dose data, but have unclear physical significance. More recently, a fit to diffraction and imaging experiments suggested that the maximum tolerable dose varies as q -1 or linearly with resolution.
Solvent flows, conformation changes and lattice reordering in a cold protein crystal
When protein crystals are abruptly cooled, the unit-cell, protein and solvent-cavity volumes all contract, but the volume of bulk-like internal solvent may expand. Outflow of this solvent from the unit cell and its accumulation in defective interior crystal regions has been suggested as one cause of the large increase in crystal mosaicity on cooling. It is shown that when apoferritin crystals are abruptly cooled to temperatures between 220 and 260 K, the unit cell contracts, solvent is pushed out and the mosaicity grows.
Unusual scaling for two-dimensional avalanches: Curing the faceting and scaling in the lower critical dimension
The nonequilibrium random-field Ising model is well studied, yet there are outstanding questions. In two dimensions, power-law scaling approaches fail and the critical disorder is difficult to pin down. Additionally, the presence of faceting on the square lattice creates avalanches that are lattice dependent at small scales. We propose two methods which we find solve these issues. First, we perform large-scale simulations on a Voronoi lattice to mitigate the effects of faceting.
Multifaceted machine learning of competing orders in disordered interacting systems
While the nonperturbative interaction effects in the fractional quantum Hall regime can be readily simulated through exact diagonalization, it has been challenging to establish a suitable diagnostic that can label different phases in the presence of competing interactions and disorder. Here we introduce a multifaceted framework using a simple artificial neural network (ANN) to detect defining features of a fractional quantum Hall state, a charge-density-wave state and a localized state using the entanglement spectra and charge density as independent input.
Interacting valley Chern insulator and its topological imprint on moiré superconductors
One salient feature of systems with moiré superlattice is that the Chern number of "minibands" originating from each valley of the original graphene Brillouin zone becomes a well-defined quantized number because the miniband from each valley can be isolated from the rest of the spectrum due to the moiré potential. Then a moiré system with a well-defined valley Chern number can become a nonchiral topological insulator with U(1)×Z3 symmetry and a Z classification at the free fermion level.
Spin Seebeck Imaging of Spin-Torque Switching in Antiferromagnetic Pt/NiO Heterostructures
As electrical control of Neél order opens the door to reliable antiferromagnetic spintronic devices, understanding the microscopic mechanisms of antiferromagnetic switching is crucial. Spatially resolved studies are necessary to distinguish multiple nonuniform switching mechanisms; however, progress has been hindered by the lack of tabletop techniques to image the Neél order. We demonstrate spin Seebeck microscopy as a sensitive tabletop method for imaging antiferromagnetism in thin films and apply this technique to study spin-torque switching in Pt/NiO and Pt/NiO/Pt heterostructures.
Spatial control of heavy-fermion superconductivity in CeIrIn5
Although crystals of strongly correlated metals exhibit a diverse set of electronic ground states, few approaches exist for spatially modulating their properties. In this study, we demonstrate disorder-free control, on the micrometer scale, over the superconducting state in samples of the heavy-fermion superconductor CeIrIn5. We pattern crystals by focused ion beam milling to tailor the boundary conditions for the elastic deformation upon thermal contraction during cooling.
Light-Induced Surface Potential Modification in MoS2 Monolayers on Au Nanostripe Arrays
In this work, the surface potential (VS) of exfoliated MoS2 monolayers on Au nanostripe arrays with period of 500 nm was investigated using Kelvin probe force microscopy. The surface morphology showed that the suspended MoS2 region between neighboring Au stripes underwent tensile-strain. In the dark, the VS of the MoS2 region on the Au stripe (VS-Au) was larger than that of the suspended MoS2 region (VS-S). However, under green light illumination, VS-Au became smaller than VS-S.
Erratum: Spin Hall torques generated by rare-earth thin films [Phys. Rev. B <b>95</b> , 064412 (2017)]
Equation (4) in the original paper contains an incorrect factor of α in the second term of the numerator. The correct equation should be as follows: (Formula Presented). This is a purely typographical error and does not affect any other part of the paper or the analysis. We thank Professor A. Manchon for bringing this error to our attention. © 2019 American Physical Society.