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Evidence of high-temperature exciton condensation in two-dimensional atomic double layers

Cornell Affiliated Author(s)
Author
Z. Wang
D.A. Rhodes
K. Watanabe
T. Taniguchi
J.C. Hone
J. Shan
K.F. Mak
Abstract

A Bose–Einstein condensate is the ground state of a dilute gas of bosons, such as atoms cooled to temperatures close to absolute zero1. With much smaller mass, excitons (bound electron–hole pairs) are expected to condense at considerably higher temperatures2–7. Two-dimensional van der Waals semiconductors with very strong exciton binding are ideal systems for the study of high-temperature exciton condensation. Here we study electrically generated interlayer excitons in MoSe2–WSe2 atomic double layers with a density of up to 1012 excitons per square centimetre.

Journal
Nature
Date Published
Funding Source
DE-SC0013883
DE-SC0019481
DMR-1420634
JPMJCR15F3
Group (Lab)
Jie Shan Group
Kin Fai Mak Group

Characterization of a Fast-Framing X-Ray Camera with Wide Dynamic Range for High-Energy Imaging

Cornell Affiliated Author(s)
Author
K.S. Shanks
H.T. Philipp
J.T. Weizeorick
M. Hammer
M.W. Tate
P. Purohit
A. Miceli
Sol Gruner
Abstract

We present first characterization results, with a focus on high-flux measurements, of a fast-framing, wide-dynamic-range x-ray camera intended for high-energy imaging. The MM-PAD-2.1 uses an integrating pixel front-end with a charge removal architecture and in-pixel counter to extend the pixel well depth while maintaining low read noise across the full dynamic range. The charge-removal mechanism is dead-time-less (i.e., incoming signal continues to be integrated by the front-end while charge removal is taking place).

Conference Name
.
Date Published
Funding Source
DE-SC0016035
DE-SC0017631
Group (Lab)
Sol M. Gruner Group

Preparation of Macroscopic Block-Copolymer-Based Gyroidal Mesoscale Single Crystals by Solvent Evaporation

Cornell Affiliated Author(s)
Author
E.M. Susca
P.A. Beaucage
R.P. Thedford
A. Singer
Sol Gruner
L.A. Estroff
U. Wiesner
Abstract

Properties arising from ordered periodic mesostructures are often obscured by small, randomly oriented domains and grain boundaries. Bulk macroscopic single crystals with mesoscale periodicity are needed to establish fundamental structure–property correlations for materials ordered at this length scale (10–100 nm). A solvent-evaporation-induced crystallization method providing access to large (millimeter to centimeter) single-crystal mesostructures, specifically bicontinuous gyroids, in thick films (>100 µm) derived from block copolymers is reported.

Journal
Advanced Materials
Date Published
Funding Source
DMR-1332208
DMR-1719875
DE-SC0017631
DMR-1707836
1719875
DGE-1650441
BES
DE-SC0010560
Group (Lab)
Sol M. Gruner Group

Synergistic Coordination of Chromatin Torsional Mechanics and Topoisomerase Activity

Cornell Affiliated Author(s)
Author
T.T. Le
X. Gao
S.H. Park
J. Lee
J.T. Inman
J.H. Lee
J.L. Killian
R.P. Badman
J.M. Berger
M.D. Wang
Abstract

The material properties of eukaryotic chromatin fibers partition supercoiling ahead of progressing replication forks, illustrating that chromatin provides a buffer against torsional stress and that its unique mechanical properties help to facilitate replication and minimize genome instability. © 2019 Elsevier Inc. DNA replication in eukaryotes generates DNA supercoiling, which may intertwine (braid) daughter chromatin fibers to form precatenanes, posing topological challenges during chromosome segregation. The mechanisms that limit precatenane formation remain unclear.

Journal
Cell
Date Published
Research Area
Group (Lab)
Michelle Wang Group

Electronic and vibrational signatures of ruthenium vacancies in Sr2RuO4 thin films

Cornell Affiliated Author(s)
Author
G. Kim
Y.E. Suyolcu
J. Herrero-Martin
D. Putzky
H.P. Nair
J.P. Ruf
N.J. Schreiber
C. Dietl
G. Christiani
G. Logvenov
M. Minola
P.A. Van Aken
K.M. Shen
D.G. Schlom
B. Keimer
Abstract

The synthesis of stoichiometric Sr2RuO4 thin films has been a challenge because of the high volatility of ruthenium oxide precursors, which gives rise to ruthenium vacancies in the films. Ru vacancies greatly affect the transport properties and electronic phase behavior of Sr2RuO4, but their direct detection is difficult due to their atomic dimensions and low concentration. We applied polarized X-ray absorption spectroscopy at the oxygen K edge and confocal Raman spectroscopy to Sr2RuO4 thin films synthesized under different conditions.

Journal
Physical Review Materials
Date Published
Funding Source
823717a-ESTEEM3
DMR-1539918
DGE-1650441
GBMF3850
669550
823717–ESTEEM3
Com4Com
Group (Lab)
Kyle Shen Group

Probing and controlling magnetic states in 2D layered magnetic materials

Cornell Affiliated Author(s)
Author
Kin Mak
Jie Shan
Daniel Ralph
Abstract

The discovery of atomic monolayer magnetic materials has triggered significant interest in the magnetism/spintronics and 2D van der Waals materials communities. Here we review recent progress in this rapidly growing field. We survey the physical properties of the large class of layered magnetic materials, and discuss recent advances in the study of these materials in the 2D limit.

Journal
Springer Science and Business Media LLC
Date Published
Funding Source
DMR-1719875
1719875
Group (Lab)
Jie Shan Group
Kin Fai Mak Group

Using Acoustic Perturbations to Dynamically Tune Shear Thickening in Colloidal Suspensions

Cornell Affiliated Author(s)
Author
P. Sehgal
M. Ramaswamy
Itai Cohen
B.J. Kirby
Abstract

Colloidal suspensions in industrial processes often exhibit shear thickening that is difficult to control actively. Here, we use piezoelectric transducers to apply acoustic perturbations to dynamically tune the suspension viscosity in the shear-thickening regime. We attribute the mechanism of dethickening to the disruption of shear-induced force chains via perturbations that are large relative to the particle roughness scale.

Journal
Physical Review Letters
Date Published
Funding Source
1U54CA210184-01
NNCI-1542081
1232666
1509308
1804963
Research Area
Group (Lab)
Itai Cohen Group

Capillary Origami with Atomically Thin Membranes

Cornell Affiliated Author(s)
Author
M.F. Reynolds
K.L. McGill
M.A. Wang
H. Gao
F. Mujid
K. Kang
J. Park
M.Z. Miskin
Itai Cohen
P.L. McEuen
Abstract

Small-scale optical and mechanical components and machines require control over three-dimensional structure at the microscale. Inspired by the analogy between paper and two-dimensional materials, origami-style folding of atomically thin materials offers a promising approach for making microscale structures from the thinnest possible sheets. In this Letter, we show that a monolayer of molybdenum disulfide (MoS2) can be folded into three-dimensional shapes by a technique called capillary origami, in which the surface tension of a droplet drives the folding of a thin sheet.

Journal
Nano Letters
Date Published
Funding Source
DMR-1719875
DMR-1539918
NSF DMR-1420709
1719875
NNCI-1542081
FA9550-16-1-0031
DGE-1746045
DMR-1757420
Research Area
Group (Lab)
Itai Cohen Group
Paul McEuen Group

Long valley lifetime of dark excitons in single-layer WSe2

Cornell Affiliated Author(s)
Author
Y. Tang
K.F. Mak
J. Shan
Abstract

Single-layer transition metal dichalcogenides provide a promising material system to explore the electron’s valley degree of freedom as a quantum information carrier. The valley degree of freedom can be directly accessed by means of optical excitation. However, rapid valley relaxation of optically excited electron-hole pairs (excitons) through the exchange interaction has been a major roadblock. Theoretically such valley relaxation is suppressed in dark excitons, suggesting a potential route for long valley lifetimes.

Journal
Nature Communications
Date Published
Funding Source
DE-SC0019481
-SC0019481
DESC0013883
Group (Lab)
Jie Shan Group
Kin Fai Mak Group