Skip to main content

Publications

Influence of Strain on the Surface-Oxygen Interaction and the Oxygen Evolution Reaction of SrIrO3

Cornell Affiliated Author(s)
Author
D.-Y. Kuo
C.J. Eom
J.K. Kawasaki
G. Petretto
J.N. Nelson
G. Hautier
E.J. Crumlin
K.M. Shen
D.G. Schlom
J. Suntivich
Abstract

Understanding how physicochemical properties of materials affect the oxygen evolution reaction (OER) has enormous scientific and technological implications for the OER electrocatalyst design. We present our investigation on the role of strain on the surface-oxygen interaction and the OER on well-defined single-termination SrIrO3 films. Our approach employs a combination of molecular-beam epitaxy, electrochemical characterizations, ambient-pressure X-ray photoelectron spectroscopy, and density functional theory (DFT).

Journal
Journal of Physical Chemistry C
Date Published
Funding Source
29120589
DMR-1120296
ECCS-0335765
DE-AC02-05CH11231
DE-SC-SC0018029
2.5020.11
Group (Lab)
Kyle Shen Group

Quantitative light microscopy of dense suspensions: Colloid science at the next decimal place

Cornell Affiliated Author(s)
Author
B.D. Leahy
N.Y.C. Lin
Itai Cohen
Abstract

Since the days of Perrin (1908) [1], microscopy methods have played an important role in the study of colloidal suspensions. Along with the continued development of new imaging techniques, colloid scientists have also implemented a sophisticated range of computational analyses. These analysis techniques are often the unsung heroes that hold the promise of unlocking scientific mysteries at the next decimal place of colloid science.

Journal
Current Opinion in Colloid and Interface Science
Date Published
Funding Source
1509308
CBET-1509308
DMR-1507607
56046-ND7
Group (Lab)
Itai Cohen Group

Strong Enhancement of the Spin Hall Effect by Spin Fluctuations near the Curie Point of FexPt1-x Alloys

Cornell Affiliated Author(s)
Author
Y. Ou
D.C. Ralph
Robert Buhrman
Abstract

Robust spin Hall effects (SHE) have recently been observed in nonmagnetic heavy metal systems with strong spin-orbit interactions. These SHE are either attributed to an intrinsic band-structure effect or to extrinsic spin-dependent scattering from impurities, namely, side jump or skew scattering. Here we report on an extraordinarily strong spin Hall effect, attributable to spin fluctuations, in ferromagnetic FexPt1-x alloys near their Curie point, tunable with x.

Journal
Physical Review Letters
Date Published
Funding Source
ECCS-1542081
1542081
DMR-1120296
10.13039/100000006
N000014-15-1-2449

Realizing the Haldane Phase with Bosons in Optical Lattices

Cornell Affiliated Author(s)
Author
J. Xu
Q. Gu
E.J. Mueller
Abstract

We analyze an experimentally realizable model of bosons in a zigzag optical lattice, showing that, by rapidly modulating the magnetic field, one can tune interaction parameters and realize an analog of the Haldane phase. We explain how quantum gas microscopy can be used to detect this phase's nonlocal string order and its topological edge states. We model the detection process. We also find that this model can display supersolid correlations, but argue that they only occur at parameter values which would be challenging to realize in an experiment. © 2018 American Physical Society.

Journal
Physical Review Letters
Date Published
Funding Source
10.13039/501100001809
11504021
11574028
10.13039/100000001
PHY-1508300
11504021
11574028
PHY-1508300

Spin–Orbit Torques in NbSe/Permalloy Bilayers

Cornell Affiliated Author(s)
Author
Marcos Guimarães
Gregory Stiehl
David MacNeill
Neal Reynolds
Daniel Ralph
Abstract

We present measurements of current-induced spin-orbit torques generated by NbSe2, a fully metallic transition-metal dichalcogenide material, made using the spin-torque ferromagnetic resonance (ST-FMR) technique with NbSe2/Permalloy bilayers. In addition to the out-of-plane Oersted torque expected from current flow in the metallic NbSe2 layer, we also observe an in-plane antidamping torque with torque conductivity σS ? 103 (?/2e)(?m)?1 and indications of a weak field-like contribution to the out-of-plane torque oriented opposite to the Oersted torque.

Journal
American Chemical Society (ACS)
Date Published
Funding Source
Rubicon 680-50-1311
1144153
1406333
1542081
1708499
1719875
DMR-1406333
DMR-1708499
W911NF-15-1-0447
DGE-1144153
DMR-1719875
ECCS-1542081

Lieb-Schultz-Mattis theorem and its generalizations from the perspective of the symmetry-protected topological phase

Cornell Affiliated Author(s)
Author
Chao-Ming Jian
Zhen Bi
Cenke Xu
Abstract

We ask whether a local Hamiltonian with a featureless (fully gapped and nondegenerate) ground state could exist in certain quantum spin systems. We address this question by mapping the vicinity of certain quantum critical point (or gapless phase) of the d-dimensional spin system under study to the boundary of a (d+1)-dimensional bulk state, and the lattice symmetry of the spin system acts as an onsite symmetry in the field theory that describes both the selected critical point of the spin system and the corresponding boundary state of the (d+1)-dimensional bulk.

Journal
Physical Review B
Date Published
Funding Source
1151208
Group (Lab)
Chao-Ming Jian Group

Non-Abelian fermionization and fractional quantum Hall transitions

Cornell Affiliated Author(s)
Author
A. Hui
M. Mulligan
Eun-Ah Kim
Abstract

There has been a recent surge of interest in dualities relating theories of Chern-Simons gauge fields coupled to either bosons or fermions within the condensed matter community, particularly in the context of topological insulators and the half-filled Landau level. Here, we study the application of one such duality to the long-standing problem of quantum Hall interplateaux transitions.

Journal
Physical Review B
Date Published
Group (Lab)

Strongly Interaction-Enhanced Valley Magnetic Response in Monolayer WSe2

Cornell Affiliated Author(s)
Author
Z. Wang
K.F. Mak
J. Shan
Abstract

We measure the doping dependence of the valley Zeeman splitting of the fundamental optical transitions in monolayer WSe2 under an out-of-plane magnetic field by optical reflection contrast and photoluminescence spectroscopy. A nonlinear valley Zeeman effect, correlated with an over fourfold enhancement in the g factor, is observed. The effect occurs when the Fermi level crosses the spin-split upper conduction band, corresponding to a change of the spin-valley degeneracy from two to four. The enhancement increases and shows no sign of saturation as the sample temperature decreases.

Journal
Physical Review Letters
Date Published
Funding Source
10.13039/100000001
DMR-1420451
DMR-1420451
DESC0012635
DESC0013883
Group (Lab)
Jie Shan Group
Kin Fai Mak Group

Micropattern differentiation of mouse pluripotent stem cells recapitulates embryo regionalized cell fate patterning

Cornell Affiliated Author(s)
Author
S.M. Morgani
J.J. Metzger
J. Nichols
E.D. Siggia
A.-K. Hadjantonakis
Abstract

During gastrulation epiblast cells exit pluripotency as they specify and spatially arrange the three germ layers of the embryo. Similarly, human pluripotent stem cells (PSCs) undergo spatially organized fate specification on micropatterned surfaces. Since in vivo validation is not possible for the human, we developed a mouse PSC micropattern system and, with direct comparisons to mouse embryos, reveal the robust specification of distinct regional identities.

Journal
eLife
Date Published
Funding Source
PHY1502151
R01HD080699
P30CA008748
R01DK084391
C029568
Research Area

Efficient switching of 3-terminal magnetic tunnel junctions by the giant spin Hall effect of Pt85Hf15 alloy

Cornell Affiliated Author(s)
Author
Minh-Hai Nguyen
Shengjie Shi
Graham Rowlands
Sriharsha Aradhya
Colin Jermain
D. Ralph
Robert Buhrman
Abstract

Recent research has indicated that introducing impurities that increase the resistivity of Pt can enhance the efficiency of the spin Hall torque it generates. Here, we directly demonstrate the usefulness of this strategy by fabricating prototype 3-terminal in-plane-magnetized magnetic tunnel junctions that utilize the spin Hall torque from a Pt85Hf15 alloy and measuring the critical currents for switching.

Journal
AIP Publishing
Date Published
Funding Source
DMR-1719875
1542081
1719875
W911NF-14-C0089
ECCS-1542081