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Publications

Irrelevance of magnetic proximity effect to spin-orbit torques in heavy-metal/ferromagnet bilayers

Cornell Affiliated Author(s)
Author
L.J. Zhu
D.C. Ralph
Robert Buhrman
Abstract

The magnetic proximity effect (MPE) is a well-established magnetic phenomenon that occurs at certain heavy-metal (HM)/ferromagnet (FM) interfaces. However, there is still an active debate as to whether the presence of a MPE affects spin transport through such a HM/FM interface. Here we demonstrate that the MPE at Pt/Co and Au0.25Pt0.75/Co interfaces can be enhanced substantially by thermal annealing protocols.

Journal
Physical Review B
Date Published
Funding Source
N00014-15-1-2449

Fast, reliable spin-orbit-torque switching in three terminal magnetic tunnel junctions with Hf dusting layer

Cornell Affiliated Author(s)
Author
Robert Buhrman
Shengjie Shi
Yongxi Ou
Daniel Ralph
Abstract

Since the discovery of the large spin Hall effect in certain heavy metals, there has been continuous interest in utilizing this spin-orbit torque (SOT) effect in constructing a non-volatile memory that can be switched by an electric current. The key to future application of this type of memory is achieving both a short write time and a low write current, which will lower the energy cost compared to existing and other emerging memory technologies.

Conference Name
Conference
Date Published
Funding Source
W911NF-14-C0089
DMR-1120296
ECCS-0335765

Highly Efficient Spin-Current Generation by the Spin Hall Effect in Au1-xPtx

Cornell Affiliated Author(s)
Author
L. Zhu
D.C. Ralph
Robert Buhrman
Abstract

We report very efficient spin-current generation by the spin Hall effect in the alloy Au0.25Pt0.75, which, as determined by two different direct spin-orbit torque measurements, exhibits a giant internal spin Hall ratio of ≥0.58 (antidamping spin-orbit torque efficiency of approximately 0.35 in bilayers with Co), a relatively low resistivity of approximately 83 μΩ cm, an exceptionally large spin Hall conductivity of ≥7.0×105Ω-1m-1, and a spin diffusion length of 1.7 nm.

Journal
Physical Review Applied
Date Published
Funding Source
W911NF-14-C0089
DMR-1719875
ECCS-1542081
N00014-15-1-2449

Structural, magnetic, and transport properties of Fe1- xRhx/MgO(001) films grown by molecular-beam epitaxy

Cornell Affiliated Author(s)
Author
A.B. Mei
Y. Tang
J.L. Grab
J. Schubert
D.C. Ralph
D.G. Schlom
Abstract

Fe1- xRhx layers are grown with varying rhodium fraction x on (001)-oriented MgO substrates by molecular-beam epitaxy. Film structural, morphological, magnetic, and transport properties are investigated. At room temperature, layers are ferromagnetic (FM) for x < 0.48 and antiferromagnetic (AF) for x > 0.48. Separating the two magnetically ordered phases at x = 0.48 is an abrupt change in the Fe1- xRhx lattice parameter of Δa = 0.0028 nm (Δa/a =-0.9%). For AF layers, the FM state is recovered by heating across a first-order phase transition.

Journal
Applied Physics Letters
Date Published
Funding Source
1740286
ECCS-1740136
2758.001
2758.003

Reorientable Spin Direction for Spin Current Produced by the Anomalous Hall Effect

Cornell Affiliated Author(s)
Author
J.D. Gibbons
D. Macneill
Robert Buhrman
D.C. Ralph
Abstract

We show experimentally that the spin direction of the spin current generated by spin-orbit interactions within a ferromagnetic layer can be reoriented by turning the magnetization direction of this layer. We do this by measuring the fieldlike component of spin-orbit torque generated by an exchange-biased Fe95Gd5 thin film and acting on a nearby Co40Fe40B20 layer. The relative angle of the Co40Fe40B20 and Fe95Gd5 magnetic moments is varied by applying an external magnetic field.

Journal
Physical Review Applied
Date Published

Creation of localized skyrmion bubbles in Co/Pt bilayers using a spin-valve nanopillar

Cornell Affiliated Author(s)
Author
J.L. Grab
A.E. Rugar
D.C. Ralph
Abstract

We fabricate devices in which a magnetic nanopillar spin valve makes contact to a Co/Pt bilayer thin film with perpendicular magnetic anisotropy, to achieve local control of domains in the Co/Pt bilayer underneath the nanopillar. The goal is to develop the ability to nucleate, detect, and annihilate magnetic skyrmions in the Co/Pt using spin-polarized currents from the nanopillar. We demonstrate the ability to distinguish the local behavior of the Co/Pt film beneath the nanopillar from the extended film and show that the two can switch independently of each other.

Journal
Physical Review B
Date Published
Funding Source
ECCS-1542081
DMR-1120296
DMR-1719875

Strong Enhancement of the Spin Hall Effect by Spin Fluctuations near the Curie Point of FexPt1-x Alloys

Cornell Affiliated Author(s)
Author
Y. Ou
D.C. Ralph
Robert Buhrman
Abstract

Robust spin Hall effects (SHE) have recently been observed in nonmagnetic heavy metal systems with strong spin-orbit interactions. These SHE are either attributed to an intrinsic band-structure effect or to extrinsic spin-dependent scattering from impurities, namely, side jump or skew scattering. Here we report on an extraordinarily strong spin Hall effect, attributable to spin fluctuations, in ferromagnetic FexPt1-x alloys near their Curie point, tunable with x.

Journal
Physical Review Letters
Date Published
Funding Source
ECCS-1542081
1542081
DMR-1120296
10.13039/100000006
N000014-15-1-2449

Spin–Orbit Torques in NbSe/Permalloy Bilayers

Cornell Affiliated Author(s)
Author
Marcos Guimarães
Gregory Stiehl
David MacNeill
Neal Reynolds
Daniel Ralph
Abstract

We present measurements of current-induced spin-orbit torques generated by NbSe2, a fully metallic transition-metal dichalcogenide material, made using the spin-torque ferromagnetic resonance (ST-FMR) technique with NbSe2/Permalloy bilayers. In addition to the out-of-plane Oersted torque expected from current flow in the metallic NbSe2 layer, we also observe an in-plane antidamping torque with torque conductivity σS ? 103 (?/2e)(?m)?1 and indications of a weak field-like contribution to the out-of-plane torque oriented opposite to the Oersted torque.

Journal
American Chemical Society (ACS)
Date Published
Funding Source
Rubicon 680-50-1311
1144153
1406333
1542081
1708499
1719875
DMR-1406333
DMR-1708499
W911NF-15-1-0447
DGE-1144153
DMR-1719875
ECCS-1542081

Efficient switching of 3-terminal magnetic tunnel junctions by the giant spin Hall effect of Pt85Hf15 alloy

Cornell Affiliated Author(s)
Author
Minh-Hai Nguyen
Shengjie Shi
Graham Rowlands
Sriharsha Aradhya
Colin Jermain
D. Ralph
Robert Buhrman
Abstract

Recent research has indicated that introducing impurities that increase the resistivity of Pt can enhance the efficiency of the spin Hall torque it generates. Here, we directly demonstrate the usefulness of this strategy by fabricating prototype 3-terminal in-plane-magnetized magnetic tunnel junctions that utilize the spin Hall torque from a Pt85Hf15 alloy and measuring the critical currents for switching.

Journal
AIP Publishing
Date Published
Funding Source
DMR-1719875
1542081
1719875
W911NF-14-C0089
ECCS-1542081

Lewis-Acid-Catalyzed Interfacial Polymerization of Covalent Organic Framework Films

Cornell Affiliated Author(s)
Author
Michio Matsumoto
Lauren Valentino
Gregory Stiehl
Halleh Balch
Amanda Corcos
Feng Wang
Daniel Ralph
Benito Mariñas
William Dichtel
Abstract

Covalent organic frameworks (COFs) are crystalline polymers with covalent bonds in two or three dimensions, providing pores 1–5 nm in diameter. COFs are typically isolated as microcrystalline powders, which are unsuitable for many applications that would leverage their tunable structures, such as optoelectronic devices and nanofiltration membranes. Here, we report the interfacial polymerization of polyfunctional amine and aldehyde monomers with a Lewis acid catalyst, Sc(OTf)3. Immiscible solutions segregate the catalyst from the monomers, confining polymerization to the solution interface.

Journal
Elsevier BV
Date Published
Funding Source
DMR-1719875
W911NF-15-1-0447
1706219
DMR-1332208
CBET-1706219