Publications
Imaging Dirac-mass disorder from magnetic dopant atoms in the ferromagnetic topological insulator Crx(Bi0.1Sb0.9)2-xTe3
To achieve and use the most exotic electronic phenomena predicted for the surface states of 3D topological insulators (TIs), it is necessary to open a "Dirac-mass gap" in their spectrum by breaking timereversal symmetry. Use of magnetic dopant atoms to generate a ferromagnetic state is the most widely applied approach. However, it is unknown how the spatial arrangements of the magnetic dopant atoms influence the Dirac-mass gap at the atomic scale or, conversely, whether the ferromagnetic interactions between dopant atoms are influenced by the topological surface states.
A microfabricated fixed path length silicon sample holder improves background subtraction for cryoSAXS
The application of small-angle X-ray scattering (SAXS) for high-throughput characterization of biological macromolecules in solution is limited by radiation damage. By cryocooling samples, radiation damage and required sample volumes can be reduced by orders of magnitude. However, the challenges of reproducibly creating the identically sized vitrified samples necessary for conventional background subtraction limit the widespread adoption of this method. Fixed path length silicon sample holders for cryoSAXS have been microfabricated to address these challenges.
Identifying the 'fingerprint' of antiferromagnetic spin fluctuations in iron pnictide superconductors
Cooper pairing in the iron-based high-T c superconductors is often conjectured to involve bosonic fluctuations. Among the candidates are antiferromagnetic spin fluctuations and d-orbital fluctuations amplified by phonons. Any such electron-boson interaction should alter the electron's 'self-energy', and then become detectable through consequent modifications in the energy dependence of the electron's momentum and lifetime.
Evidence for a small hole pocket in the Fermi surface of underdoped YBa2Cu3Oy
In underdoped cuprate superconductors, the Fermi surface undergoes a reconstruction that produces a small electron pocket, but whether there is another, as yet, undetected portion to the Fermi surface is unknown. Establishing the complete topology of the Fermi surface is key to identifying the mechanism responsible for its reconstruction. Here we report evidence for a second Fermi pocket in underdoped YBa2Cu3Oy, detected as a small quantum oscillation frequency in the thermoelectric response and in the c-axis resistance.
Breaking of Valley Degeneracy by Magnetic Field in Monolayer MoSe2
Using polarization-resolved photoluminescence spectroscopy, we investigate the breaking of valley degeneracy by an out-of-plane magnetic field in back-gated monolayer MoSe2 devices. We observe a linear splitting of -0.22meV/T between luminescence peak energies in σ+ and σ- emission for both neutral and charged excitons. The optical selection rules of monolayer MoSe2 couple the photon handedness to the exciton valley degree of freedom; so this splitting demonstrates valley degeneracy breaking.
Black phosphorus nanoelectromechanical resonators vibrating at very high frequencies
We report on the experimental demonstration of a new type of nanoelectromechanical resonator based on black phosphorus crystals. Facilitated by a highly efficient dry transfer technique, crystalline black phosphorus flakes are harnessed to enable drumhead resonators vibrating at high and very high frequencies (HF and VHF bands, up to ∼100 MHz). We investigate the resonant vibrational responses from the black phosphorus crystals by devising both electrical and optical excitation schemes, in addition to measuring the undriven thermomechanical motions in these suspended nanostructures.
Spatially resolved transient dynamics of charge density waves in NbSe3
We have developed methods for acquiring temporally and spatially resolved spectrograms of the velocity of sliding charge-density waves (CDWs), allowing unprecedented access to CDW dynamics. Complex transients arising from the interplay between elastic and plastic processes occur when the driving field direction is reversed. A transient spectral component due to shear elasticity can be unambiguously identified, and allows the most direct determination to date of the CDW's shear elastic modulus.
Interplay of spin-orbit interactions, dimensionality, and octahedral rotations in semimetallic SrIrO3
We employ reactive molecular-beam epitaxy to synthesize the metastable perovskite SrIrO3 and utilize in situ angle-resolved photoemission to reveal its electronic structure as an exotic narrow-band semimetal. We discover remarkably narrow bands which originate from a confluence of strong spin-orbit interactions, dimensionality, and both in- and out-of-plane IrO6 octahedral rotations.
Kinetics of Bose-Einstein condensation in a dimple potential
We model the dynamics of condensation in a bimodal trap, consisting of a large reservoir region, and a tight "dimple" whose depth can be controlled. Experimental investigations have found that such dimple traps provide an efficient means of achieving condensation. In our kinetic equations, we include two- and three-body processes. The two-body processes populate the dimple, and lead to loss when one of the colliding atoms is ejected from the trap. The three-body processes produce heating and loss.
Determination of crystallographic intensities from sparse data
X-ray serial microcrystallography involves the collection and merging of frames of diffraction data from randomly oriented protein microcrystals. The number of diffracted X-rays in each frame is limited by radiation damage, and this number decreases with crystal size. The data in the frame are said to be sparse if too few X-rays are collected to determine the orientation of the microcrystal. It is commonly assumed that sparse crystal diffraction frames cannot be merged, thereby setting a lower limit to the size of microcrystals that may be merged with a given source fluence.