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Publications

Effective Spin-Mixing Conductance of Heavy-Metal–Ferromagnet Interfaces

Cornell Affiliated Author(s)
Author
Lijun Zhu
Daniel Ralph
Robert Buhrman
Abstract

The effective spin-mixing conductance (Geff↑↓) of a heavy-metal-ferromagnet (HM-FM) interface characterizes the efficiency of the interfacial spin transport. Accurately determining Geff↑↓ is critical to the quantitative understanding of measurements of direct and inverse spin Hall effects. Geff↑↓ is typically ascertained from the inverse dependence of magnetic damping on the FM thickness under the assumption that spin pumping is the dominant mechanism affecting this dependence.

Journal
American Physical Society (APS)
Date Published
Funding Source
1542081
1719875

Variation of the giant intrinsic spin Hall conductivity of Pt with carrier lifetime

Cornell Affiliated Author(s)
Author
Lijun Zhu
Lujun Zhu
Manling Sui
Daniel Ralph
Robert Buhrman
Abstract

More than a decade after the first theoretical and experimental studies of the spin Hall conductivity (SHC) of Pt, both its dominant origin and amplitude remain in dispute. We report the experimental determination of the rapid variation of the intrinsic SHC of Pt with the carrier lifetime (t) in the dirty-metal regime by incorporating finely dispersed MgO intersite impurities into the Pt, while maintaining its essential band structure.

Journal
American Association for the Advancement of Science (AAAS)
Date Published
Funding Source
ECCS-1542081
DMR-1719875
1542081
1719875
N00014-15-1-2449
W911NF-14-C0089
GK201903024
2019JQ-433

Self-assembly and properties of domain walls in BiFeO3 layers grown via molecular-beam epitaxy

Cornell Affiliated Author(s)
Author
Antonio Mei
Yongjian Tang
Jürgen Schubert
Debdeep Jena
Huili Xing
Daniel Ralph
Darrell Schlom
Abstract

Bismuth ferrite layers, ∼200-nm-thick, are deposited on SrRuO3-coated DyScO3(110)o substrates in a step-flow growth regime via adsorption-controlled molecular-beam epitaxy. Structural characterization shows the films to be phase pure with substrate-limited mosaicity (0.012° x-ray diffraction ω-rocking curve widths). The film surfaces are atomically smooth (0.2 nm root-mean-square height fluctuations) and consist of 260-nm-wide [11̄1]o-oriented terraces and unit-cell-tall (0.4 nm) step edges.

Journal
AIP Publishing
Date Published
Funding Source
ECCS 1740286
2758.003
1338010

Exceptionally High, Strongly Temperature Dependent, Spin Hall Conductivity of SrRuO

Cornell Affiliated Author(s)
Author
Yongxi Ou
Zhe Wang
Celesta Chang
Hari Nair
Hanjong Paik
Neal Reynolds
Daniel Ralph
David Muller
Darrell Schlom
Robert Buhrman
Abstract

Spin-orbit torques (SOT) in thin film heterostructures originate from strong spin-orbit interactions (SOI) that, in the bulk, generate a spin current due either to extrinsic spin-dependent, skew, or/and side-jump scattering or to intrinsic Berry curvature in the conduction bands. While most SOT studies have focused on materials with heavy metal components, the oxide perovskite SrRuO3 has been predicted to have a pronounced Berry curvature.

Journal
American Chemical Society (ACS)
Date Published
Funding Source
DMR-1719875
ECCS-1542081
DE-SC0002334

Enhancing Spin-Orbit Torque by Strong Interfacial Scattering From Ultrathin Insertion Layers

Cornell Affiliated Author(s)
Author
Lijun Zhu
Lujun Zhu
Shengjie Shi
Manling Sui
D.C. Ralph
Robert Buhrman
Abstract

Increasing dampinglike spin-orbit torque (SOT) is of fundamental importance for enabling new research into spintronics phenomena and also technologically urgent for advancing low-power spin-torque memory, logic, and oscillator devices. Here, we demonstrate that enhancing interfacial scattering by inserting ultrathin layers within spin Hall metals with intrinsic or side-jump mechanisms can significantly enhance the spin Hall ratio.

Journal
American Physical Society (APS)
Date Published
Funding Source
DMR-1719875
2019JQ-433
N00014-15-1-2449
GK201903024
W911NF-14-C0089
ECCS-1542081

Enhancement of spin transparency by interfacial alloying

Cornell Affiliated Author(s)
Author
Lijun Zhu
Daniel Ralph
Robert Buhrman
Abstract

We report that atomic-layer alloying (intermixing) at a Pt/Co interface can increase, by approximately 30%, rather than degrade the interfacial spin transparency, and thereby strengthen the efficiency of the dampinglike spin-orbit torque arising from the spin Hall effect in the Pt. At the same time, this interfacial alloying substantially reduces fieldlike spin-orbit torque.

Journal
American Physical Society (APS)
Date Published
Funding Source
DMR-1719875
1719875
ECCS-1542081
N00014-15-1-2449

Strong damping-like spin-orbit torque and tunable Dzyaloshinskii-Moriya interaction generated by low-resistivity Pd1−xPtx alloys

Cornell Affiliated Author(s)
Author
Lijun Zhu
Kemal Sobotkiewich
Xin Ma
Xiaoqin Li
Daniel Ralph
Robert Buhrman
Abstract

Despite their great promise for providing a pathway for very efficient and fast manipulation of magnetization, spin-orbit torque (SOT) operations are currently energy inefficient due to a low damping-like SOT efficiency per unit current bias, and/or the very high resistivity of the spin Hall materials. This work reports an advantageous spin Hall material, Pd 1− x Pt x , which combines a low resistivity with a giant spin Hall effect as evidenced with three independent SOT ferromagnetic detectors.

Journal
Wiley
Date Published
Funding Source
DE-SC0012670
DMR-1719875
ECCS-1542081
N00014-15-1-2449
W911NF-14-C0089

Spin-Orbit Torques in Heavy-Metal-Ferromagnet Bilayers with Varying Strengths of Interfacial Spin-Orbit Coupling

Cornell Affiliated Author(s)
Author
L. Zhu
D.C. Ralph
Robert Buhrman
Abstract

Despite intense efforts it has remained unresolved whether and how interfacial spin-orbit coupling (ISOC) affects spin transport across heavy-metal (HM)-ferromagnet (FM) interfaces. Here we report conclusive experiment evidence that the ISOC at HM/FM interfaces is the dominant mechanism for "spin memory loss". An increase in ISOC significantly reduces, in a linear manner, the dampinglike spin-orbit torque (SOT) exerted on the FM layer via degradation of the spin transparency of the interface for spin currents generated in the HM.

Journal
Physical Review Letters
Date Published
Funding Source
W911NF-14-C0089
ECCS-1542081

Current-Induced Torques with Dresselhaus Symmetry Due to Resistance Anisotropy in 2D Materials

Cornell Affiliated Author(s)
Author
Gregory Stiehl
David MacNeill
Nikhil Sivadas
Ismail Baggari
Marcos Guimarães
Neal Reynolds
Lena Kourkoutis
Craig Fennie
Robert Buhrman
Daniel Ralph
Abstract

We report measurements of current-induced torques in heterostructures of Permalloy (Py) with TaTe2, a transition-metal dichalcogenide (TMD) material possessing low crystal symmetry, and observe a torque component with Dresselhaus symmetry. We suggest that the dominant mechanism for this Dresselhaus component is not a spin-orbit torque but rather the Oersted field arising from a component of current that flows perpendicular to the applied voltage due to resistance anisotropy within the TaTe2.

Journal
American Chemical Society (ACS)
Date Published
Funding Source
Rubicon 680-50-1311
DE-SC0017671
1429155
1542081
1708499
1719875
DMR-1539918
DMR-1708499
DMR-1719875
ECCS-1542081
NSF-MRI-1429155
680-50-1311

Vector-resolved magnetooptic kerr effect measurements of spin-orbit torque

Cornell Affiliated Author(s)
Author
Halise Celik
H. Kannan
T. Wang
A.R. Mellnik
X. Fan
X. Zhou
R. Barri
D.C. Ralph
M.F. Doty
V.O. Lorenz
J.Q. Xiao
Abstract

We demonstrate simultaneous detection of current-driven dampinglike and fieldlike spin-orbit torques in heavy metal/ferromagnetic metal bilayers by measuring all three magnetization components mx,my, and mz using a vector-resolved magnetooptic Kerr effect (MOKE) technique based on quadrant detection. We investigate the magnitude and direction of spin-orbit torques in a series of platinum/permalloy samples, finding good agreement with results obtained via polar and quadratic MOKE measurements without quadrant detection. © 1965-2012 IEEE.

Journal
IEEE Transactions on Magnetics
Date Published
Funding Source
1624976
DMR-1624976
DE-SC0016380