Spectroscopic indications of polaronic behavior of the strong spin-orbit insulator Sr3Ir2O7
Abstract
We investigate the bilayer Ruddlesden-Popper iridate Sr3Ir 2O7 by temperature-dependent angle-resolved photoemission. At low temperatures, we find a fully gapped correlated insulator, characterized by a small charge gap and narrow bandwidths. The low-energy spectral features show a pronounced temperature-dependent broadening and non-quasiparticle-like Gaussian line shapes. Together, these spectral features provide experimental evidence for a polaronic ground state. We observe similar behavior for the single-layer cousin Sr2IrO4, indicating that strong electron-boson coupling dominates the low-energy excitations of this exotic family of 5d compounds. © 2013 American Physical Society.
Date Published
Journal
Physical Review B - Condensed Matter and Materials Physics
Volume
87
Issue
24
URL
https://www.scopus.com/inward/record.uri?eid=2-s2.0-84879934007&doi=10.1103%2fPhysRevB.87.241106&partnerID=40&md5=4a5e1ed754b39909b260c7433190394d
DOI
10.1103/PhysRevB.87.241106
Research Area
Group (Lab)
Kyle Shen Group
Funding Source
EP/I031014/1
24224010