The role of electron-phonon interactions on the coherence lifetime of monolayer transition metal dichalcogenides
Abstract
We investigate the excitonic dephasing of transition metal dichalcogenides, namely MoS2, MoSe2 and WSe2 atomic monolayer thick and bulk crystals, in order to understand the factors that determine the optical coherence in these materials. Coherent nonlinear optical spectroscopy, temperature dependent absorption combined with theoretical calculations of the phonon spectra, reveal the important role electron-phonon interactions plat in dephasing process. The temperature dependence of the electronic band gap and the excitonic linewidth combined with 'ab initio' calculations of the phonon energies and the phonon density of state reveal strong interaction with the E' and E" phonon modes.
Date Published
Conference Name
Journal of Physics: Conference Series
Publisher
IOP Publishing
URL
https://www.scopus.com/inward/record.uri?eid=2-s2.0-85028764793&doi=10.1088%2f1742-6596%2f864%2f1%2f012035&partnerID=40&md5=9cb8949f3f30f833219bb90ef009d1f3
DOI
10.1088/1742-6596/864/1/012035
Research Area
Group (Lab)
Jie Shan Group
Funding Source
1434897
ACI-1053575
54075-ND10
DE-SC0012635